Elu U. et al. «Seven‑octave high‑brightness and carrier‑envelope‑phase‑stable light source» (Nature Photonics, 2021)
1. Main Spectral Parameters
- Spectral range: 7 octaves — from 340 nm (ultraviolet) to 40,000 nm (40 µm, terahertz range).
- Spectrum continuity: no spectral gaps across the entire range.
- Carrier‑envelope phase (CEP) stability:
- root‑mean‑square (RMS) deviation of fluctuations — less than 300 mrad;
- phase stability maintained across the full spectrum (from UV to THz).
- Brightness: 2–5 orders of magnitude higher than synchrotron sources in the IR range.
- Spectral power density:
- in the UV range (340–450 nm): comparable to pump power in the mid‑IR;
- at 3200 nm: peak intensity up to 2,5 MW;
- in the THz range (up to 40,000 nm): intensity of 1,8 MW, 15 dB/nm below the pump level.
- Coherence: high spatial and temporal coherence across the entire spectrum.
2. Pulse Parameters
- Pulse duration: sub‑cycle, less than 3 optical cycles.
- Central wavelength: 3200 nm (3,2 µm).
- Repetition rate: 160 kHz.
- Average power: 2,8 W.
- Pulse energy: 31 nJ.
- Peak power:
- in the UV range: up to 2,5 MW (at 35 bar pressure);
- in the THz range: 1,8 MW (at 20 bar pressure).
- Intensity: up to TW/cm2 in both UV and THz ranges.
- Pulse shape: controllable, with tunability via gas pressure adjustment in the fibre.
3. System Components and Their Parameters
3.1. Seed Source
- Type: fibre optical parametric chirped‑pulse amplifier (OPCPA) in the mid‑IR range.
- Pump wavelength: 3,2 µm.
- Operation mode: pulsed, with passive CEP stabilisation.
- Output radiation parameters:
- pulse duration: 94 fs;
- repetition rate: 160 kHz;
- average power: 2,8 W.
3.2. Microstructured Fibre (ARR‑PCF)
- Fibre type: anti‑resonant reflection photonic‑crystal fibre (Anti‑Resonant Reflection Photonic‑Crystal Fibre, ARR‑PCF).
- Length: 20 cm.
- Core diameter: 92 µm.
- Coupling efficiency: 93%.
- Construction: the fibre is placed inside a gas cell with CaF2 windows (3 mm thick).
- Internal medium: argon (Ar) at adjustable pressure.
- Functions:
- soliton self‑compression of the pulse;
- dispersive wave (DW) generation;
- spectral broadening via nonlinear effects (self‑phase modulation, etc.).
3.3. Nonlinear Crystal
- Composition: BaGa2GeSe6 (BGGSe).
- Thickness: 2,6 mm.
- Process: intra‑pulse difference frequency generation (IP‑DFG).
- IP‑DFG efficiency: up to 2% under optimal conditions.
- Advantages:
- high nonlinear susceptibility;
- broad transparency in the mid‑IR and THz ranges;
- compatibility with high peak power.
3.4. CEP Stabilisation System
- Method: active feedback loop for carrier‑envelope phase control.
- Monitoring: electro‑optical sampling (EOS) for direct measurement of the electric field waveform.
- Stabilisation accuracy: fluctuations less than 300 mrad.
- Components:
- CEP detectors;
- control elements (piezo actuators, acousto‑optic modulators).
4. Operating Conditions and Settings
- Gas pressure in the fibre (argon): adjustable, in the range 20–35 bar:
- 25 bar — optimal dispersive wave generation and spectral broadening in the near‑IR;
- 35 bar — enhancement of the UV component (down to 340 nm), peak power of 2,5 MW in UV;
- 20 bar — spectral extension into the THz range (up to 40,000 nm), peak power of 1,8 MW.
- Energy conversion efficiency:
- into dispersive wave (at 35 bar): 0,2%, corresponding to an average power of 5 mW (31 nJ) in DW;
- overall supercontinuum generation efficiency: high due to cascaded nonlinear processes.
- Temperature regime: stable operation at room temperature, without active cooling.
5. Key Performance Metrics
- Dynamic range for spectroscopy: high, due to brightness and coherence.
- Compactness: table‑top source, requiring no large infrastructures (e.g., synchrotrons).
- Versatility: tunable spectral power distribution via gas pressure control.
- Synchronisation: low jitter between different spectral components, critical for time‑resolved measurements.
- Reliability: stable operation over long sessions (hours of continuous generation).
6. Practical Capabilities of the System
- Attosecond physics: generation of attosecond pulses from CEP‑stable mid‑IR radiation.
- Broadband spectroscopy: simultaneous analysis of molecular vibrations (IR) and electronic transitions (UV‑visible).
- Coherent control: manipulation of molecular and quantum system dynamics using synthesised pulses.
- Metrology: optical frequency combs with extended range for precision frequency measurements.
- Biophotonics and medicine: multimodal imaging (combination of UV fluorescence and IR spectroscopy).
- Materials research: study of topological materials, superconductivity, and phase transitions under strong fields.
Summary: the system represents the first compact source of CEP‑stable radiation with a 7‑octave spectral coverage, combining fibre optics, supercontinuum generation, and parametric amplification. Its key advantages are high brightness, stability, and the ability to tune the spectrum for specific applications.