Elu U. et al. «Seven‑octave high‑brightness and carrier‑envelope‑phase‑stable light source» (Nature Photonics, 2021)

1. Main Spectral Parameters

  • Spectral range: 7 octaves — from 340 nm (ultraviolet) to 40,000 nm (40 µm, terahertz range).
  • Spectrum continuity: no spectral gaps across the entire range.
  • Carrier‑envelope phase (CEP) stability:
  • root‑mean‑square (RMS) deviation of fluctuations — less than 300 mrad;
  • phase stability maintained across the full spectrum (from UV to THz).
  • Brightness: 2–5 orders of magnitude higher than synchrotron sources in the IR range.
  • Spectral power density:
  • in the UV range (340–450 nm): comparable to pump power in the mid‑IR;
  • at 3200 nm: peak intensity up to 2,5 MW;
  • in the THz range (up to 40,000 nm): intensity of 1,8 MW, 15 dB/nm below the pump level.
  • Coherence: high spatial and temporal coherence across the entire spectrum.

2. Pulse Parameters

  • Pulse duration: sub‑cycle, less than 3 optical cycles.
  • Central wavelength: 3200 nm (3,2 µm).
  • Repetition rate: 160 kHz.
  • Average power: 2,8 W.
  • Pulse energy: 31 nJ.
  • Peak power:
  • in the UV range: up to 2,5 MW (at 35 bar pressure);
  • in the THz range: 1,8 MW (at 20 bar pressure).
  • Intensity: up to TW/cm2 in both UV and THz ranges.
  • Pulse shape: controllable, with tunability via gas pressure adjustment in the fibre.

3. System Components and Their Parameters

3.1. Seed Source

  • Type: fibre optical parametric chirped‑pulse amplifier (OPCPA) in the mid‑IR range.
  • Pump wavelength: 3,2 µm.
  • Operation mode: pulsed, with passive CEP stabilisation.
  • Output radiation parameters:
  • pulse duration: 94 fs;
  • repetition rate: 160 kHz;
  • average power: 2,8 W.

3.2. Microstructured Fibre (ARR‑PCF)

  • Fibre type: anti‑resonant reflection photonic‑crystal fibre (Anti‑Resonant Reflection Photonic‑Crystal Fibre, ARR‑PCF).
  • Length: 20 cm.
  • Core diameter: 92 µm.
  • Coupling efficiency: 93%.
  • Construction: the fibre is placed inside a gas cell with CaF2​ windows (3 mm thick).
  • Internal medium: argon (Ar) at adjustable pressure.
  • Functions:
  • soliton self‑compression of the pulse;
  • dispersive wave (DW) generation;
  • spectral broadening via nonlinear effects (self‑phase modulation, etc.).

3.3. Nonlinear Crystal

  • Composition: BaGa2​GeSe6​ (BGGSe).
  • Thickness: 2,6 mm.
  • Process: intra‑pulse difference frequency generation (IP‑DFG).
  • IP‑DFG efficiency: up to 2% under optimal conditions.
  • Advantages:
  • high nonlinear susceptibility;
  • broad transparency in the mid‑IR and THz ranges;
  • compatibility with high peak power.

3.4. CEP Stabilisation System

  • Method: active feedback loop for carrier‑envelope phase control.
  • Monitoring: electro‑optical sampling (EOS) for direct measurement of the electric field waveform.
  • Stabilisation accuracy: fluctuations less than 300 mrad.
  • Components:
  • CEP detectors;
  • control elements (piezo actuators, acousto‑optic modulators).

4. Operating Conditions and Settings

  • Gas pressure in the fibre (argon): adjustable, in the range 20–35 bar:
  • 25 bar — optimal dispersive wave generation and spectral broadening in the near‑IR;
  • 35 bar — enhancement of the UV component (down to 340 nm), peak power of 2,5 MW in UV;
  • 20 bar — spectral extension into the THz range (up to 40,000 nm), peak power of 1,8 MW.
  • Energy conversion efficiency:
  • into dispersive wave (at 35 bar): 0,2%, corresponding to an average power of 5 mW (31 nJ) in DW;
  • overall supercontinuum generation efficiency: high due to cascaded nonlinear processes.
  • Temperature regime: stable operation at room temperature, without active cooling.

5. Key Performance Metrics

  • Dynamic range for spectroscopy: high, due to brightness and coherence.
  • Compactness: table‑top source, requiring no large infrastructures (e.g., synchrotrons).
  • Versatility: tunable spectral power distribution via gas pressure control.
  • Synchronisation: low jitter between different spectral components, critical for time‑resolved measurements.
  • Reliability: stable operation over long sessions (hours of continuous generation).

6. Practical Capabilities of the System

  • Attosecond physics: generation of attosecond pulses from CEP‑stable mid‑IR radiation.
  • Broadband spectroscopy: simultaneous analysis of molecular vibrations (IR) and electronic transitions (UV‑visible).
  • Coherent control: manipulation of molecular and quantum system dynamics using synthesised pulses.
  • Metrology: optical frequency combs with extended range for precision frequency measurements.
  • Biophotonics and medicine: multimodal imaging (combination of UV fluorescence and IR spectroscopy).
  • Materials research: study of topological materials, superconductivity, and phase transitions under strong fields.

Summary: the system represents the first compact source of CEP‑stable radiation with a 7‑octave spectral coverage, combining fibre optics, supercontinuum generation, and parametric amplification. Its key advantages are high brightness, stability, and the ability to tune the spectrum for specific applications.

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